Fragmentation Control of a Polyatomic Molecule by fully determined Laser-Fields
1 Photonics Institute, Vienna University of Technology, A-1040 Vienna, Austria
2 Institute of Optics and Quantum Electronics, D-07743 Jena, Germany
3 Institute of Theoretical Physics, Vienna University of Technology, A-1040 Vienna, Austria
4 Department of Physics and Astronomy, Vanderbilt University, Nashville, Tennessee 37235, USA
5 Department of Chemistry, School of Science, The University of Tokyo, Tokyo 113-0033, Japan
6 State Key Laboratory on Integrated Optoelectronics, Changchun 130012, China
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Strong-field control of acetylene fragmentation by fully determined few-cycle laser pulses is demonstrated. The control mechanism is shown to be based on electron recollision and inelastic ionization from inner-valence molecular orbitals.
© Owned by the authors, published by EDP Sciences, 2013
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