Two-Dimensional Electronic Spectroscopy of a Model Dimer System
1 Institute for Optical Sciences and Departments of Chemistry and Physics, University of Toronto, 80 St. George Street, Toronto, Ontario M5S 3H6, Canada.
2 Department of Chemistry and Biochemistry, University of Regina, 3737 Wascana Parkway, Regina, SK, S4S 0A2, Canada.
3 Max Planck Research Department for Structural Dynamics, Department of Physics, University of Hamburg, Centre for Free Electron Laser Science, DESY, Notkestrasse 85, D-22607 Hamburg, Germany.
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Two-dimensional spectra of a dimer were measured to determine the timescale for electronic decoherence at room temperature. Anti-correlated beats in the crosspeaks were observed only during the period corresponding to the measured homogeneous lifetime.
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